Production of Bitumen Modified with Low-Molecular Organic Compounds from Petroleum Residues. 3. Tar Modified with Formaldehyde

2021;
: pp. 608–620
1
Lviv Polytechnic National University
2
Lviv Polytechnic National University
3
Institute of Chemistry and Chemical Technology Lviv Polytechnic National University
4
Lviv Polytechnic National University
5
Lviv Polytechnic National University, Danylo Halytsky Lviv National Medical University
6
Lviv Polytechnic National University
7
Lviv Polytechnic National University, Ukraine
8
Lviv Polytechnic National University

The chemical modification of tar with formaldehyde as 37% aqueous solutionhas been studied in the presence of the catalysts. Hydrochloric acid, sulfuric acid, sodium hydroxide and acid tar were used as the catalysts. The effect of the catalyst nature and amount, as well as temperature, process time and initial components ratio on the softening point, penetration, brittle point and adhesion to crushed stone has been determined. The structure of the modified tars was confirmed by IR spectroscopy. The structural-group composition was determined. Arene-formaldehyde resins have been synthesized on the basis of toluene and modified tars using hydrochloric acid as a catalyst. The synthesized resins were characterized using IR spectroscopy. The chemistry of the tar modification with formaldehyde has been proposed.

  1. McNally T. (Ed): Polymer Modified Bitumen. Properties and Characterization. Woodhead Publ., 2011. https://doi.org/10.1533/9780857093721
  2. Pyshyev S., Gunka V., Grytsenko Yu. et al.: Chem. Chem. Technol., 2016, 10, 631. https://doi.org/10.23939/chcht10.04si.631
  3. Grynyshyn O., Bratychak M., Krynytskiy V. et al.: Chem. Chem. Technol., 2008, 2, 47. https://doi.org/10.23939/chcht02.01.047
  4. Bratychak M., Chervinskyy T., Astakhova O. et al.: Chem. Chem. Technol., 2010, 4, 325. https://doi.org/10.23939/chcht04.04.325
  5. Bratychak M., Grynyshyn O., Astakhova O. et al.: Ecol. Chem. Eng. S, 2010, 17, 309.
  6. Bratychak M., Grynyshyn O., Prysiazhnyi Yu., Pushak A.: Naftopolimerni Smoly iz Funktsiinymy Grupamy. Syntez, Vlastyvosti, Zastosuvannia. Monografia. Vyd-vo Lviv Polytechnic, Lviv 2016.
  7. Ivashkiv O., Astakhova O., Shyshchak O. et al.: Chem. Chem. Technol., 2015, 9, 69. https://doi.org/10.23939/chcht09.01.069
  8. Bratychak M., Iatsyshyn O., Shyshchak O. et al.: Chem. Chem. Technol., 2017, 11, 49. https://doi.org/10.23939/chcht11.01.049
  9. Bratychak M., Shyshchak O., Astakhova O., Ivashkiv O.: Oligomers with Functional Groups Based on Epoxy Resins. Synthesis, Properties and Application. Lviv Polytechnic Publ. House, Lviv 2019.
  10. Strap G., Astakhova O., Lazorko O. et al.: Chem. Chem. Technol., 2013, 7, 279.https://doi.org/10.23939/chcht07.03.279
  11. Astakhova O., Shved M., Zubal O. et al.: Chem. Chem. Technol., 2019, 13, 112. https://doi.org/10.23939/chcht13.01.112
  12. Sidun Yu., Solodkyy S., Shved M. et al.: Chem. Chem. Technol., 2019, 13, 489.https://doi.org/10.23939/chcht13.04.489
  13. Bratychak M., Shyshchak O., Astakhova O., Gunka V.: Oligomers Based on Cyclic Compounds. Synthesis, Properties and Application. Lviv Polytechnic Publ. House, Lviv 2021.
  14. Gunka V., Prysiazhnyi Yu., Hrynchuk Yu. et al.: Chem. Chem. Technol., 2021, 15, 443. https://doi.org/10.23939/chcht15.03.443
  15. Bratychak M., Gunka V., Prysiazhnyi Yu. et al.: Chem. Chem. Technol., 2021, 15, 274.https://doi.org/10.23939/chcht15.02.274
  16. Gunka V., Demchuk Y., Sidun I. et al.: Pet. Coal, 2020, 62, 420.
  17. Bratychak M., Gunka V.: Khimia nafty i gazu. Vyd-vo Lviv Polytechnic, Lviv 2017.
  18. http://online.budstandart.com/ua/catalog/doc-page.html?id_doc=79270.
  19. Gunka V., Demchuk Y., Sidun I. et al.: Road Mater. Pavement Des., 2020. https://doi.org/10.1080/14680629.2020.1808518
  20. http://online.budstandart.com/ua/catalog/doc-page.html?id_doc=78305
  21. Demchuk Y., Gunka V., Pyshyev S. et al.: Chem. Chem. Technol., 2020, 14, 251. https://doi.org/10.23939/chcht14.02.251
  22. Gun R. Neftianye Bitumy. Khimia, Moskva 1973.
  23. Moshchinskaia N.: Polimernye Materialy na Osnove Aromaticheskikh Uglevodorodov i Formaldegida. Monografia. Tekhnika, Kiev 1969.
  24. Bratychak M., Gunka V.: Khimia Nafty i Gazu. Vyd-vo Lviv Polytechnic, Lviv 2020.
  25. Knop A., Sheib B.: Fenolnye Smoly i Materialy na ikh Osnovie. Khimia, Moskva 1983.
  26. Gutsuliak V., Nevskii V., Safronova A.: Arenformaldegidnye Oligomery. Nauka 1986.
  27. Nesmeianov A., Nesmeianov N.: Nachala Organicheskoi Khimii. T. 2. Moskva 1969.
  28. Kazitsyna L., Kupletskaia N.: Primenenie UF-, IK- i IaMR-Spektroskopii v Organicheskoi Khimii. Vysshaia shkola. Moskva 1971.